CN103478894B - There is the camellia extract composition of pungent note and the application in cigarette thereof - Google Patents
There is the camellia extract composition of pungent note and the application in cigarette thereof Download PDFInfo
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Abstract
There is a camellia extract composition for pungent note, and said composition is as the application of cigarette additive in cigarette.Described camellia extract composition, is formed by tea flower extract and pungent fragrant flavor confect.Add in cigarette provided by the invention there is the camellia extract composition of pungent note after, make cigarette flavor harmony, improve the distinctive fragrance of tobacco leaf, increase pungent note, make the more lush nature of cigarette perfume (or spice), promote the rich of cigarette flavor, make the more lush nature of cigarette perfume (or spice), improve the solid sense of cigarette flavor, increase the mellow and full property of cigarette flavor, person experiences naturally easily to bring cigarette smoking, and assorted gas, stimulation reduce, and overall sucking quality is improved.
Description
Technical field
The invention belongs to tobacco spice technical field, relate to and a kind of there is the camellia extract composition of pungent note and the application in cigarette thereof.
Background technology
Essence and flavoring agent is widely used in the fields such as tobacco, food, daily use chemicals, and natural perfume material due to its composition complicated, fragrance enriches, fragrance remaining time is the indispensable raw material of preparing essence lastingly.
International tobacco business pays much attention to the development and application of essence spice for cigarette, and the technology of production application high-quality essence and flavoring agent is used as the core technology of oneself.Along with tobacco business technological progress and greatly develop the proposition of Chinese-style cigarette target, essence spice for cigarette technology as the important core technology of tobacco business, as one of formation Chinese-style cigarette quality characteristic, the key making Chinese-style cigarette core technology.Essence and flavoring agent can give the style and features of cigarette product uniqueness, improves the suction quality of cigarette product, is one of important connotation of constructing Chinese-style cigarette core competitiveness.Still there is certain deficiency in current domestic cigarette product, the Application and Development of novel essence spice for cigarette is an important solution route in style and features and suction quality etc.
There is abundant natural perfume material resource in China, about has more than 500 to plant fragrant plant and is distributed widely in 20 provinces and cities, but only have minority to be exploited, and there is the problems such as level of processing is low, application technology is single.
Tea tree (Camellia sinensis) is Theaceae Camellia Plants, and its cultivation has had history in thousand, and in China, distributed pole is wide.Tea Flower is very abundant as the accessory substance resource in Tea Production process.Tea Flower has the advantages that the florescence is long, the amount of blooming is large and fragrance is fresh and sweet, has high value of exploiting and utilizing.In recent years, the comprehensive utilization of Tea Flower is more and more paid attention to.
Tea Flower is rich in multiple beneficial composition and the active materials such as protein, Tea Polyphenols, tea polysaccharide, Tea Saponin, flavonoids, amino acid, vitamin, trace element and superoxide dismutase (SOD), theobromine, has hypoglycemic, reducing blood lipid, anticoagulant, antithrombotic, nourishing, beauty treatment and the effect such as anticancer.Containing number of chemical material and fragrance component in Tea Flower.The fragrance component of Tea Flower is mainly alcohols, ester class, aldehydes and lower alkyl hydrocarbons, and wherein the relative amount of acetophenone, 2-enanthol, phthalic acid two (2-ethylhexyl) ester, linalool is higher.The Tea flower essence fragrance prepared by tea flower extract is fresh and clean, and sweet spiciness is strongly fragrant, has higher potential using value.
Pungent spices with the fresh and sweet rhythm of the fragrance of a flower, the pungent sweet and clear dense warm fragrance of a flower, head perfume has the gentle fresh banksia rose and Xin Xiang, end rhythm have sweet and in the fragrance of a flower and cream fragrant, dense and lasting.Pungent spices has makes a perfumed ribbon have feeling of freshness, natural sense, and in mediation essence, fragrance comparatively rushes thick raw material fragrance, can make overall fragrance flavouring, and make its many rhythm.
Have no at present by tea flower extract and the flavor compositions of Xin Xiang flavor confect and the application in cigarette thereof.
Goal of the invention of the present invention is to provide a kind of camellia extract composition with pungent note, and said composition is as the application of cigarette additive in cigarette, for improving sucking quality and the sense organ comfort level of cigarette.
Summary of the invention
Inventor adopts tea flower extract to be primary raw material, adds and has the pungent spices of the natural equivalent composition of stronger hamony (as clove bud oil, ginger oil, extract of cinnamomum cassia bark, eugenol, coriander extract, fennel seeds wet goods) formulated to Tea Flower.Said composition elegant fragrance nature, fresh many rhythms, graceful breath with pungent note.
A first aspect of the present invention provides a kind of camellia extract composition, formed by tea flower extract and pungent fragrant flavor confect, wherein said pungent spices be selected from that carrot seed oil, clove bud oil, aniseed oil, ennel oil, ginger oil, coriander extract, cumal, β-China pink are rare, one or more in eugenol, sage clary oil, radix valerianae extract, extract of cinnamomum cassia bark, radix tarxaci extract.
Composition described according to a first aspect of the present invention, wherein said tea flower extract is selected from Tea Flower medicinal extract, essential oil of the flower of Camellia sinensis, Tea Flower absolute oil, Tea Flower tincture or its combination.
Composition described according to a first aspect of the present invention, in a specific embodiment, wherein said pungent spices is that clove bud oil, ennel oil, coriander extract, β-China pink are rare, eugenol and extract of cinnamomum cassia bark.
Composition described according to a first aspect of the present invention, the preparation method of wherein said Tea Flower medicinal extract, Tea Flower absolute oil and/or Tea Flower tincture comprises the step of raw material Tea Flower being carried out to ultra high pressure extraction.
Composition described according to a first aspect of the present invention, in a specific embodiment, the preparation method of described Tea Flower tincture, Tea Flower medicinal extract and/or Tea Flower absolute oil, comprises following step (1), step (1)-(2) or step (1)-(3):
(1) ultra high pressure extraction: take a certain amount of Tea Flower and put into ultra high pressure extraction tank, add the edible alcohol of at least 2 times of (w/w) Tea Flower weight, carry out ultra high pressure extraction, obtain Tea Flower tincture 1, the concentration of wherein said edible alcohol is 20-70%(mass concentration); Preferably, 1/5-1/10 Tea Flower tincture 1 being concentrated into original volume obtains Tea Flower tincture 2;
(2) Tea Flower medicinal extract is prepared: the Tea Flower tincture 1 obtained in step (1) or Tea Flower tincture 2 are concentrated further, obtain Tea Flower medicinal extract;
(3) Tea Flower absolute oil is prepared: the Tea Flower medicinal extract obtained with a certain amount of 95% ethanol resuspension step (2), then freezing processing (such as-10 DEG C to-20 DEG C) is carried out, cooling time is that 16-48h(is preferably 20-36h) then filter, concentrated, obtain Tea Flower absolute oil.
In the present invention, freezing temperature can be-10 DEG C to-20 DEG C.
In a specific embodiment, in the preparation method of above-mentioned Tea Flower medicinal extract, Tea Flower absolute oil and/or Tea Flower tincture, in step (1), described for adopted Tea Flower be Tea Flower fresh flower, dried flower, spray Ethanol Treatment Tea Flower, saline sook Tea Flower or alcohol immersion Tea Flower.
In a specific embodiment, in the preparation method of above-mentioned Tea Flower medicinal extract, Tea Flower absolute oil and/or Tea Flower tincture, in step (1), add the edible alcohol of at least 2-15 times of (w/w) Tea Flower weight, be preferably 2-10 doubly, 2-8 doubly, 3-8 doubly (w/w), be more preferably 4-7 doubly (w/w), such as 4 times, 5 times, 6 times or 7 times (w/w).
In a specific embodiment, in the preparation method of above-mentioned Tea Flower tincture, Tea Flower medicinal extract and/or Tea Flower absolute oil, in step (1), particularly, the concentration of described edible alcohol is 20-70%(mass concentration), 20-40%, 20-50%, 40-50%, 50-70%, 20%, 30%, 40%, 50%, 60%, 70%.
In a specific embodiment, in the preparation method of above-mentioned Tea Flower medicinal extract, Tea Flower absolute oil and/or Tea Flower tincture, in step (1), release immediately after ultra high pressure extraction.
In a specific embodiment, in the preparation method of above-mentioned Tea Flower tincture, Tea Flower medicinal extract and/or Tea Flower absolute oil, in step (1), the pressure of described super-pressure is 150-500Mpa; Particularly, be 150-250Mpa, 150-300Mpa, 250-300Mpa, 250-350Mpa, 250-500Mpa, 300-350Mpa, 300-500Mpa, 350-500Mpa, 150Mpa, 200Mpa, 250Mpa, 300Mpa, 350Mpa, 400Mpa, 450Mpa, 500Mpa etc.
In a specific embodiment, in the preparation method of above-mentioned Tea Flower tincture, Tea Flower medicinal extract and/or Tea Flower absolute oil, in step (1), dwell time is 5-120min, be preferably 5-60min, be more preferably 10-30min, such as 10-15min, 10-20min, 10-25min, 15-20min, 15-25min, 15-30min, 20-25min, 20-30min, 25-30min, 10min, 15min, 20min, 25min, 30min etc.
In a specific embodiment, in the preparation method of above-mentioned Tea Flower medicinal extract, Tea Flower absolute oil and/or Tea Flower tincture, concentrated in step (1) or (2) can be the method that those skilled in the art know, such as suction filtration concentrates.
Composition described according to a first aspect of the present invention, in a specific embodiment, the preparation method of wherein said essential oil of the flower of Camellia sinensis is the reduced steam way of distillation.
Composition described according to a first aspect of the present invention, in a specific embodiment, the preparation method of described essential oil of the flower of Camellia sinensis, comprises the steps:
(1) taking a certain amount of Tea Flower loads in the decompression extraction element being furnished with trapping cold-trap;
(2) add the water of Tea Flower weight at least 5 times, and the temperature of the water added is more than 80 DEG C, at least 5min is soaked in sealing, is cooled to 30-70 DEG C;
(3-1) carry out reduced steam distillation, temperature used is identical with cooled temperature in step (2), and vacuum is 1-17kpa, collects distillate;
Preferably, also comprise step (3-2): repeat operation 1 time in step (2) and (3-1) or repeatedly, and merge distillate;
(4) in using, low polar organic solvent carries out 1 time the distillate obtained in step (3-1) or step (3-2) or repeatedly back extraction (such as 2,3,4 or 5 times, preferably 3 times), obtains stripping workshop; Stripping workshop is concentrated, obtains concentrate;
(5) use concentrate weight 2-4 absolute ethyl alcohol doubly to carry out backwash to the concentrate obtained in step (4), during reduced pressure concentration removing wherein remains, after low polar organic solvent, obtain essential oil of the flower of Camellia sinensis.
In a specific embodiment, in the preparation method of above-mentioned essential oil of the flower of Camellia sinensis, for adopted Tea Flower is Tea Flower fresh flower, dried flower, spray Ethanol Treatment Tea Flower, saline sook Tea Flower or alcohol immersion Tea Flower described in step (1).
In a specific embodiment, in the preparation method of above-mentioned essential oil of the flower of Camellia sinensis, the amount of the water added in step (2) is 5-50 times of Tea Flower weight, be preferably 5-40 times or 8-40 times, be more preferably 10-30 doubly, such as 10-15 doubly, 10-20 doubly, 10-25 doubly, 15-20 doubly, 15-25 doubly, 15-30 doubly, 20-25 doubly, 20-30 doubly, 10 times, 11 times, 12 times, 13 times, 14 times, 15 times, 16 times, 17 times, 18 times, 19 times, 20 times, 21 times, 22 times, 23 times, 24 times, 25 times, 26 times, 27 times, 28 times, 29 times or 30 times.
In a specific embodiment, in the preparation method of above-mentioned essential oil of the flower of Camellia sinensis, the temperature of the water added in step (2) is preferably more than 85 DEG C, is more preferably more than 90 DEG C, more preferably more than 95 DEG C, such as 95 DEG C, 96 DEG C, 97 DEG C, 98 DEG C, 99 DEG C, preferably 100 DEG C; Particularly preferably, the water added is boiling water.Soak and carry out at ambient pressure, the temperature of the boiling water of immersion is generally 100 DEG C, and those skilled in the art know, according to atmospheric difference, boiling point is different.
In a specific embodiment, in the preparation method of above-mentioned essential oil of the flower of Camellia sinensis, the time that in step (2), sealing is soaked is 5min-4h, be preferably 5min-4h, 5min-3h or 5min-2h, be more preferably 5-60min, 5-50min or 5-40min, be particularly preferably 5-30min, such as 5-18min, 5-20min, 5-25min or 18-30min.
In a specific embodiment, in the preparation method of above-mentioned essential oil of the flower of Camellia sinensis, step is cooled to 30-70 DEG C in (2), such as 30-40 DEG C, 30-50 DEG C, 30-60 DEG C, 40-50 DEG C, 45-55 DEG C, 40-60 DEG C, 40-70 DEG C, 50-60 DEG C, 50-70 DEG C or 60-70 DEG C.
Those skilled in the art know, and vacuum and vapo(u)rizing temperature are corresponding to a certain extent, need to guarantee to allow under to fixed temperature and vacuum the distilled water in cucurbit and aroma component steam.
Be not limited to theoretical restriction, temperature is lower, and required vacuum is less, and temperature is higher, and required vacuum is larger.The present inventor finds, when temperature is 30 DEG C, and vacuum 2.5kpa; The speed that distills less of 2.5kpa can be faster; When temperature is 70 DEG C, vacuum 17kpa; The speed that distills less of 17kpa can be faster.
Be not limited to theoretical restriction, on the other hand, under the prerequisite of temperature setting, if vacuum is too low, may bumping be caused, extraction pot liquid is gone out; If vacuum is too high, extraction pot liquid may be made to distill not out, do not have the effect of decompression distillation.Therefore, the vacuum ranges that each temperature value correspondence one is proper.
Therefore, about the vacuum of the distillation of reduced steam described in step (3-1) or (3-2), those skilled in the art can set according to the theory above selected temperature reference or this area knowledge, also with reference to vacuum ranges below, or can adjust on this basis:
Such as 1-12kPa, 1-10kPa, 1-9.5kPa, 1-9kPa, 1-8.5kPa, 1-8kPa, 1-7.5kPa or 1-7kPa, such as 2.5-7kPa, 1-2kPa, 1-3kPa, 1-4kPa, 1-5kPa, 1-6kPa, 2-3kPa, 2-4kPa, 2-5kPa, 2-6kPa, 2-7kPa, 3-4kPa, 3-5kPa, 3-6kPa, 3-7kPa, 4-5kPa, 4-6kPa, 4-7kPa, 5-6kPa, 5-7kPa, 6-7kPa, 6-12kPa, 8-12kPa, 10-12kPa, 1kPa, 2kPa, 3kPa, 4kPa, 5kPa, 6kPa, 7kPa, 8kPa, 9kPa, 10kPa, 11kPa or 12kPa.
In a specific embodiment, in the preparation method of above-mentioned essential oil of the flower of Camellia sinensis, in step (4), in described low polar organic solvent be selected from absolute ether and ethyl acetate any one; Ethyl acetate.In described, the consumption of low polar organic solvent can be the 1/4-1/3 of distillate volume.
In a specific embodiment, in the preparation method of above-mentioned essential oil of the flower of Camellia sinensis, the decompression extraction element used can be commercially available, or the preferred decompression extraction element used in the Chinese patent application (application number is 200910111996.2) that publication number is 101920127A.
In a specific embodiment, the composition described in first aspect present invention, wherein said tea flower extract is Tea Flower medicinal extract.
In a specific embodiment, the composition described in first aspect present invention, wherein the content of each component is with parts by weight, is respectively:
Tea Flower medicinal extract 10-30, is preferably 15-25 or 18-22, is more preferably 20;
Clove bud oil 0.05-0.15, is preferably 0.08-0.12 or 0.09-0.11, is more preferably 0.1;
Ennel oil 0.1-0.2, is preferably 0.12-0.18 or 0.13-0.16, is more preferably 0.15;
Coriander extract 0.02-0.08, is preferably 0.03-0.07 or 0.04-0.06, is more preferably 0.05;
The rare 0.05-0.15 of β-China pink, is preferably 0.08-0.12 or 0.09-0.11, is more preferably 0.1;
Eugenol 0.1-0.3, is preferably 0.15-0.25 or 0.18-0.22, is more preferably 0.2;
Extract of cinnamomum cassia bark 0.2-0.3, is preferably 0.22-0.28 or 0.24-0.26, is more preferably 0.25.
In a specific embodiment, the composition described in first aspect present invention, wherein said pungent spices is carrot seed oil, aniseed oil, ginger oil, sage clary oil, radix valerianae extract, extract of cinnamomum cassia bark, radix tarxaci extract.
In a specific embodiment, the composition described in first aspect present invention, wherein said tea flower extract is essential oil of the flower of Camellia sinensis.
In a specific embodiment, the composition described in first aspect present invention, wherein the content of each component is with parts by weight, is respectively:
Essential oil of the flower of Camellia sinensis 5-15, is preferably 8-12 or 9-11, is more preferably 10;
Carrot seed oil 0.1-0.2, is preferably 0.12-0.18 or 0.13-0.16, is more preferably 0.15;
Aniseed oil 0.05-0.15, is preferably 0.08-0.12 or 0.09-0.11, is more preferably 0.1;
Ginger oil 0.02-0.08, is preferably 0.03-0.07 or 0.04-0.06, is more preferably 0.05;
Sage clary oil 0.05-0.15, is preferably 0.08-0.12 or 0.09-0.11, is more preferably 0.1;
Radix valerianae extract 0.2-0.8, is preferably 0.3-0.7 or 0.4-0.6, is more preferably 0.55;
Extract of cinnamomum cassia bark 0.2-0.3, is preferably 0.22-0.28 or 0.24-0.26, is more preferably 0.25;
Radix tarxaci extract 0.1-0.2, is preferably 0.12-0.18 or 0.13-0.16, is more preferably 0.15.
In a specific embodiment, the composition described in first aspect present invention, wherein said pungent spices is that carrot seed oil, aniseed oil, ginger oil, β-China pink are rare, radix valerianae extract, extract of cinnamomum cassia bark, radix tarxaci extract.
In a specific embodiment, the composition described in first aspect present invention, wherein said tea flower extract is Tea Flower absolute oil.
In a specific embodiment, the composition described in first aspect present invention, wherein the content of each component is with parts by weight, is respectively: Tea Flower absolute oil 15-35, is preferably 20-30 or 22-28, is more preferably 25;
Carrot seed oil 0.1-0.2, is preferably 0.12-0.18 or 0.13-0.16, is more preferably 0.15;
Aniseed oil 0.05-0.15, is preferably 0.08-0.12 or 0.09-0.11, is more preferably 0.1;
Ginger oil 0.02-0.08, is preferably 0.03-0.07 or 0.04-0.06, is more preferably 0.05;
The rare 0.1-0.2 of β-China pink, is preferably 0.12-0.18 or 0.13-0.16, is more preferably 0.15;
Radix valerianae extract 0.2-0.8, is preferably 0.3-0.7 or 0.4-0.6, is more preferably 0.55;
Extract of cinnamomum cassia bark 0.2-0.3, is preferably 0.22-0.28 or 0.24-0.26, is more preferably 0.25;
Radix tarxaci extract 0.1-0.2, is preferably 0.12-0.18 or 0.13-0.16, is more preferably 0.15.
In a specific embodiment, the composition described in first aspect present invention, wherein said pungent spices is that clove bud oil, aniseed oil, ennel oil, β-China pink are rare, sage clary oil, extract of cinnamomum cassia bark, radix tarxaci extract.
In a specific embodiment, the composition described in first aspect present invention, wherein said tea flower extract is Tea Flower tincture.
In a specific embodiment, the composition described in first aspect present invention, wherein the content of each component is with parts by weight, is respectively: Tea Flower tincture 20-40, is preferably 25-35 or 28-32, is more preferably 30;
Clove bud oil 0.02-0.08, is preferably 0.03-0.07 or 0.04-0.06, is more preferably 0.05;
Aniseed oil 0.05-0.15, is preferably 0.08-0.12 or 0.09-0.11, is more preferably 0.1;
Ennel oil 0.02-0.08, is preferably 0.03-0.07 or 0.04-0.06, is more preferably 0.05;
The rare 0.1-0.2 of β-China pink, is preferably 0.12-0.18 or 0.13-0.16, is more preferably 0.15;
Sage clary oil 0.05-0.15, is preferably 0.08-0.12 or 0.09-0.11, is more preferably 0.1;
Extract of cinnamomum cassia bark 0.1-0.2, is preferably 0.12-0.18 or 0.13-0.16, is more preferably 0.15;
Radix tarxaci extract 0.2-0.3, is preferably 0.22-0.28 or 0.24-0.26, is more preferably 0.25.
Composition according to a first aspect of the present invention described in any one, also comprise ethanol in said composition, preferably the ethanol water of 50 ~ 95%, further preferably 60 ~ 80% ethanol water, more preferably the ethanol water of 65 ~ 75%, is particularly preferably the ethanol water of 70%;
Preferably, the weight portion content of ethanol or ethanol water is 60-90, is preferably 75-80,85-90,70-75 or 65-70.
Composition described in any one of first aspect present invention can be used as cigarette additive, particularly as the purposes of cigarette flavors.The addition manner of said composition for: use ethanol or ethanol water dissolve described in composition, being mixed with perfuming dissolution homogeneity is sprayed onto in pipe tobacco, or be sprayed onto in pipe tobacco by the composition Direct Uniform containing ethanol or ethanol water, the concrete usage ratio of perfuming solution or the composition containing ethanol or ethanol water is 0.005 ~ 0.05% of tobacco quality.
A second aspect of the present invention provides the purposes of the composition of any one of first aspect present invention in cigarette, preferably as the purposes of cigarette additive, particularly preferably as the purposes of cigarette flavors;
Preferably, said composition may be used for the internal lining paper, filter stick etc. of pipe tobacco, thin slice, cigarette.
A third aspect of the present invention provides a kind of cigarette, and it comprises the composition described in any one of first aspect present invention,
Preferably, described composition is the composition containing ethanol water;
Preferably, the consumption of the described composition containing ethanol water is 0.005 ~ 0.05% of pipe tobacco weight.
Detailed Description Of The Invention
The various term used in the present invention and phrase have and well known to a person skilled in the art general sense, but have special definition in this article, are as the criterion with implication as defined herein.
In the present invention, " tea tree " in described " Tea Flower ", if not otherwise specified, refers to the plant of Theales (Theales), Theaceae (Theaceae) or Camellia (Camellis);
In one aspect of the invention, " flower " in described " Tea Flower " comprising: perianth, oecium, gynoecium.Perianth comprises: calyx (being made up of sepal), corolla (being made up of petal).The color of flower and fragrance are from corolla.Stamen comprises: filigree and flower pesticide.Gynoecium comprises: column cap, style and ovary.
In one aspect of the invention, term " Tea Flower " can be fresh flower, also can be dry flower; If do not have specified otherwise, it refers to complete Tea Flower or a part for Tea Flower; It at least comprises petal; Alternatively, one or more being selected from sepal, stamen and gynoecium are also comprised.
In the present invention, described tea flower extract, includes but not limited to: essential oil of the flower of Camellia sinensis, Tea Flower tincture, Tea Flower medicinal extract and/or Tea Flower absolute oil; Alternatively, it also comprises auxiliary material (carrier, solvent, pigment, antioxidant, anticorrisive agent, humectant, fumet etc.).
Tea Flower described in the present invention extracts can pass through normal temperature lixiviate, heating and refluxing extraction, surname extraction, ultrasound on extracting, microwave auxiliary extraction, enzyme process auxiliary extraction, accelerated solvent extraction, supercritical fluid extraction, Simultaneous distillation-extraction, steam distillation, the combination of any one or a few method of decompression distillation etc. is prepared from, also can by commercially available (such as: China of Australia reaches international fragrance (Guangzhou) Co., Ltd, Huabao Edible Essence & Condiment (Shanghai), Hangzhou Jie Min essence and flavoring agent Co., Ltd, Shenzhen GuanLiDa BoDun spice Co., Ltd).
The separation method that described Tea Flower extracts can be the combination of any one or a few method of isolated by filtration, centrifugation, UF membrane, molecular clock, column chromatography, chromatographic isolation etc.
Term " tincture " or " tincture " refer to uses certain density ethanol, lixiviate spice berry organ or exudate and secrete fragrant animal containing fragrant organ or its aroma material preparation containing some ethanol obtained containing fragrant secretion.Tincture is worth to be called " cold process tincture " under normal temperature; Tincture obtained under heated reflux condition is called " hot method tincture "." Tea Flower tincture " used in the present invention by commercially available, also can prepare by various conventional method.
In one embodiment of the invention, described " Tea Flower tincture " can prepare by the following method:
(1) described Tea Flower includes but not limited to fresh Tea Flower, dried flower, alcohol immersion process Tea Flower, spray Ethanol Treatment Tea Flower etc.;
(2) ultra high pressure extraction: take certain quantity of fresh Tea Flower and put into ultra high pressure extraction tank, adds the edible alcohol that 7 times of concentration to Tea Flower weight are 20%, carries out release immediately after ultra high pressure extraction; The pressure of described super-pressure is: 150MPa, the dwell time: 30min;
(3) namely the 1/5-1/10 being concentrated into original volume after the extract in step (2) being carried out suction filtration obtains Tea Flower tincture.
Term " essential oil ", in broad terms, essential oil refer to from spice berry and secrete fragrant animal organ to extract the general name of the volatility fragrant containing substance goods obtained through processing, in the narrow sense, essential oil only refers to the goods with steam distillation, milling process, cold grinding method or cracking process fragrant containing substance obtained from spice berry organ (as flower, leaf, branch, skin, scapus, root, fruit, seed etc.).In actual applications, normal its narrow sense of employing." essential oil of the flower of Camellia sinensis " used in the present invention by commercially available, also can prepare by various conventional method.
In one embodiment of the invention, described " essential oil of the flower of Camellia sinensis " can prepare by the following method:
(1) take certain quantity of fresh Tea Flower to load in decompression extraction element, add the boiling water of Tea Flower weight 30 times, sealing is cooled to 70 DEG C after soaking 30min;
(2) on the decompressor being furnished with trapping cold-trap, carry out reduced steam distillation, temperature is: 70 DEG C, and vacuum is: 12kpa, collects distillate;
(3) decompression distillation complete after add Tea Flower weight 25 times boiling water in extraction element, repeat decompression distillation twice according to step (3) after merge and collect liquid;
(4) add 0.3 times and collect the long-pending ethyl acetate back extraction of liquid three times, merge stripping workshop and be concentrated into 1/10 of fresh Tea Flower weight; ;
(5) essential oil of the flower of Camellia sinensis is refined: the absolute ethyl alcohol adding concentrate 3 times in step (4) carries out backwash, reduced pressure concentration remove wherein after residual ethyl acetate essential oil of the flower of Camellia sinensis.
Term " medicinal extract ", in a broad sense, medicinal extract refers to organic solvent extraction spice berry organ or its exudate (as resin, natural gum, balm), removing solvent for use and the general designation of aroma material preparation that obtains.From in the narrow sense, medicinal extract only refer to organic solvent extraction spice berry organ obtain not containing the aroma material preparation of solvent for use and moisture." Tea Flower medicinal extract " used in the present invention by commercially available, also can prepare by various conventional method.
In one embodiment of the invention, described " Tea Flower medicinal extract " can prepare by the following method:
(1) described Tea Flower includes but not limited to fresh Tea Flower, dried flower, alcohol immersion process Tea Flower, spray Ethanol Treatment Tea Flower etc.;
(2) ultra high pressure extraction: take certain quantity of fresh Tea Flower and put into ultra high pressure extraction tank, 4 times of concentration to Tea Flower weight are 40% edible alcohol, carry out release immediately after ultra high pressure extraction; The pressure of described super-pressure is: 500MPa, the dwell time: 10min;
(3) namely the 1/5-1/10 being concentrated into original volume after the extract in step (2) being carried out suction filtration obtains Tea Flower tincture;
(4) Tea Flower medicinal extract is prepared: Tea Flower medicinal extract can be obtained by concentrated for the Tea Flower tincture obtained in step (3) continuation.
Term " absolute oil ", in a broad sense, refers to the solution extracting the fragrant composition in medicinal extract, botany bar gum, balm or face cream with high concentration ethanol, through freezing processing, elimination insoluble matter, then after pressure reducing and steaming ethanol the general designation of the aroma material preparation of gained." Tea Flower absolute oil " used in the present invention by commercially available, also can prepare by various conventional method.
In one embodiment of the invention, described " Tea Flower absolute oil " can prepare by the following method:
(1) described Tea Flower includes but not limited to fresh Tea Flower, dried flower, alcohol immersion process Tea Flower, spray Ethanol Treatment Tea Flower etc.;
(2) ultra high pressure extraction: take certain quantity of fresh Tea Flower and put into ultra high pressure extraction tank, 5 times of concentration to Tea Flower weight are 70% edible alcohol, carry out release immediately after ultra high pressure extraction; The pressure of described super-pressure is: 300MPa, the dwell time: 20min;
(3) namely the 1/5-1/10 being concentrated into original volume after the extract in step (2) being carried out suction filtration obtains Tea Flower tincture;
(4) Tea Flower medicinal extract is prepared: Tea Flower medicinal extract can be obtained by concentrated for the Tea Flower tincture obtained in step (3) continuation;
(5) Tea Flower absolute oil is prepared: with a certain amount of 95% ethanol back dissolving Tea Flower medicinal extract, filter after freezing (such as-10 DEG C to-20 DEG C) 24-48h, concentrated, obtain Tea Flower absolute oil.
In the present invention, various pungent spices (such as carrot seed oil, clove bud oil, aniseed oil, ennel oil, ginger oil, coriander extract, cumal, β-China pink rare, eugenol, sage clary oil, radix valerianae extract, extract of cinnamomum cassia bark, radix tarxaci extract) all by commercially available, such as: China of Australia reaches the various pungent spices that international fragrance (Guangzhou) Co., Ltd, Huabao Edible Essence & Condiment (Shanghai), Hangzhou Jie Min essence and flavoring agent Co., Ltd, Shenzhen GuanLiDa BoDun spice Co., Ltd etc. provide.
The beneficial effect of the invention
Provided by the invention have the camellia extract composition elegant fragrance nature of pungent note, fresh many rhythms, graceful breath with pungent note, can be widely used in tobacco, food and household chemicals field etc.
Sensory evaluating smoking's result shows: add in cigarette provided by the invention there is the camellia extract composition of pungent note after, make cigarette flavor harmony, improve the distinctive fragrance of tobacco leaf, increase pungent note, make the more lush nature of cigarette perfume (or spice), promote the rich of cigarette flavor, make the more lush nature of cigarette perfume (or spice), improve the solid sense of cigarette flavor, increase the mellow and full property of cigarette flavor, person experiences naturally easily to bring cigarette smoking, and assorted gas, stimulation reduce, and overall sucking quality is improved.
The camellia extract composition with pungent note provided by the invention is joined in cigarette, do not change original performance of cigarette, do not change the original processing technology of cigarette, improve the flavouring essence quality of cigarette, and improve sucking quality and the sense organ comfort level of cigarette, therefore have more the meaning and value of actual production.
Detailed description of the invention
Below in conjunction with embodiment, embodiment of the present invention are described in detail, but it will be understood to those of skill in the art that the following example only for illustration of the present invention, and should not be considered as limiting scope of the present invention.Unreceipted actual conditions person in embodiment, the condition of conveniently conditioned disjunction manufacturer suggestion is carried out.The unreceipted production firm person of component used, being can by the conventional products of commercial acquisition.
The Tea Flower tincture used in embodiment below prepares by the following method:
(1) raw material: fresh Tie Guanyin tea plant flower, clovershrub Tea Flower, Chinese cassia tree Tea Flower or narcissus Tea Flower;
(2) ultra high pressure extraction: take certain quantity of fresh Tea Flower and put into ultra high pressure extraction tank, adds the edible alcohol that 7 times of concentration to Tea Flower weight are 20%, carries out release immediately after ultra high pressure extraction; The pressure of described super-pressure is: 150MPa, the dwell time: 30min;
(3) namely the 1/5-1/10 being concentrated into original volume after the extract in step (2) being carried out suction filtration obtains kwan-yin Tea Flower tincture, clovershrub Tea Flower tincture, Chinese cassia tree Tea Flower tincture or narcissus Tea Flower tincture.
The essential oil of the flower of Camellia sinensis used in embodiment below prepares by the following method:
(1) take certain quantity of fresh Tea Flower (fresh Tie Guanyin tea plant flower, clovershrub Tea Flower, Chinese cassia tree Tea Flower or narcissus Tea Flower) to load in decompression extraction element, add the boiling water of Tea Flower weight 30 times, sealing is cooled to 70 DEG C after soaking 30min;
(2) on the decompressor being furnished with trapping cold-trap, carry out reduced steam distillation, temperature is: 70 DEG C, and vacuum is: 12kpa, collects distillate;
(3) decompression distillation complete after add Tea Flower weight 25 times boiling water in extraction element, repeat decompression distillation twice according to step (3) after merge and collect liquid;
(4) add 0.3 times and collect the long-pending ethyl acetate back extraction of liquid three times, merge stripping workshop and be concentrated into 1/10 of fresh Tea Flower weight; ;
(5) essential oil of the flower of Camellia sinensis is refined: the absolute ethyl alcohol adding concentrate 3 times in step (4) carries out backwash, reduced pressure concentration remove wherein after residual ethyl acetate Tie Guanyin tea plant flower essential oil, clovershrub essential oil of the flower of Camellia sinensis, Chinese cassia tree essential oil of the flower of Camellia sinensis or narcissus essential oil of the flower of Camellia sinensis.
The Tea Flower medicinal extract used in embodiment below prepares by the following method:
(1) raw material: fresh Tie Guanyin tea plant flower, clovershrub Tea Flower, Chinese cassia tree Tea Flower or narcissus Tea Flower;
(2) ultra high pressure extraction: take certain quantity of fresh Tea Flower and put into ultra high pressure extraction tank, 4 times of concentration to Tea Flower weight are 40% edible alcohol, carry out release immediately after ultra high pressure extraction; The pressure of described super-pressure is: 500MPa, the dwell time: 10min;
(3) namely the 1/5-1/10 being concentrated into original volume after the extract in step (2) being carried out suction filtration obtains Tea Flower tincture;
(4) Tea Flower medicinal extract is prepared: Tie Guanyin tea plant flower concrete, clovershrub Tea Flower medicinal extract, Chinese cassia tree tea tree flower concrete or narcissus tea tree flower concrete can be obtained by concentrated for the Tea Flower tincture obtained in step (3) continuation.
The Tea Flower absolute oil used in embodiment below prepares by the following method:
(1) raw material: fresh Tie Guanyin tea plant flower, clovershrub Tea Flower, Chinese cassia tree Tea Flower or narcissus Tea Flower;
(2) ultra high pressure extraction: take certain quantity of fresh Tea Flower and put into ultra high pressure extraction tank, 5 times of concentration to Tea Flower weight are 70% edible alcohol, carry out release immediately after ultra high pressure extraction; The pressure of described super-pressure is: 300MPa, the dwell time: 20min;
(3) namely the 1/5-1/10 being concentrated into original volume after the extract in step (2) being carried out suction filtration obtains Tea Flower tincture;
(4) Tea Flower medicinal extract is prepared: Tea Flower medicinal extract can be obtained by concentrated for the Tea Flower tincture obtained in step (3) continuation;
(5) Tea Flower absolute oil is prepared: with a certain amount of 95% ethanol back dissolving Tea Flower medicinal extract, filter after freezing (such as-10 DEG C to-20 DEG C) 24-48h, concentrated, obtain Tie Guanyin tea plant extrait, clovershrub Tea Flower absolute oil, Chinese cassia tree tea tree extrait or narcissus tea tree extrait.
The ethanol used in embodiment below reaches international fragrance (Guangzhou) Co., Ltd purchased from China of Australia, SC3005; Carrot seed oil, aniseed oil, ennel oil, extract of cinnamomum cassia bark reach international fragrance (Guangzhou) Co., Ltd purchased from China of Australia; Clove bud oil, cumal, β-China pink are rare, radix tarxaci extract is purchased from Huabao Edible Essence & Condiment (Shanghai); Coriander extract, eugenol are purchased from Hangzhou Jie Min essence and flavoring agent Co., Ltd; Ginger oil, sage clary oil, radix valerianae extract are purchased from Shenzhen GuanLiDa BoDun spice Co., Ltd.
Sensory evaluating smoking's experiment below in embodiment to be smoked panel test comparison to cigarette sample by GB5606.4-2005 by the sensory evaluating smoking committee of Fujian China Tobacco Industrial Co., Ltd..Sensory Quality of Cigarette judgment criteria is as shown in Table A.
Table A Sensory Quality of Cigarette judgment criteria
Sensory evaluating smoking's inspection rule:
1, participating in the number of smokeing panel test is 13 people.
2, aesthetic quality scores employing hundred-mark system, and highest score is 100 points.
3, projects are all divided into 0.5 unit of scoring.
4, when smokeing panel test score to gloss, fragrance, harmony, assorted gas, excitant, pleasant impression six projects, each project quality reaches the requirement of respective item, then correspondingly score.
Embodiment 1:
According to the formula in table 1, each component in table 1 except 70% ethanol is mixed, prepare the camellia extract composition with pungent fragrant note.Wherein 1# composition in contrast, only containing a kind of component Tea Flower medicinal extract.
Table 1
Embodiment 1 is prepared the camellia extract composition with pungent note that obtains according to the ratio in upper table 1, add 70% ethanol water, obtain camellia extract composition ethanolic solution.The camellia extract composition ethanolic solution with pungent note obtained evenly is sprayed onto on pipe tobacco by 0.035% of pipe tobacco weight, after baking, rolls into cigarette.Wherein 0# is as blank, on pipe tobacco, only spray the ethanol water of 70%.Then carry out sensory evaluating smoking's experiment by GB5606.4-2005, comparison scoring event of smokeing panel test is in table 2.
Table 2 Sensory Quality of Cigarette inspection original record
Smoking result shows: the score of 3# and 4# composition is with to contrast 1# composition score suitable, and 2# composition score is the highest, apparently higher than control group and other groups.Relative to 1#, 3# and 4# composition, add the cigarette of 2# composition, its cigarette flavor harmony, cigarette perfume (or spice) is soft, has the skillful bent wine taste of ageing cigarette, increases soft pungent perfume (or spice) and delicate fragrance, modify and correct the fragrant natural flavor of cigarette, the breath of supplement flue-cured tobacco fragrance, assorted gas, stimulation reduce, and overall sucking quality is improved.
Embodiment 2:
According to the formula in table 3, each component in table 3 except 70% ethanol is mixed, prepare the camellia extract composition with pungent fragrant note.Wherein 1# composition in contrast, only containing a kind of component Tea Flower medicinal extract.
Table 3
Embodiment 2 is prepared the camellia extract composition with pungent note that obtains according to the ratio in upper table 3, add 70% ethanol water, obtain camellia extract composition ethanolic solution.The camellia extract composition ethanolic solution with pungent note obtained evenly is sprayed onto on pipe tobacco by 0.025% of pipe tobacco weight, after baking, rolls into cigarette.Wherein 0# is as blank, on pipe tobacco, only spray the ethanol water of 70%.Then carry out sensory evaluating smoking's experiment by GB5606.4-2005, comparison scoring event of smokeing panel test is in table 4.
Table 4 Sensory Quality of Cigarette inspection original record
Smoking result shows: the score of 3# and 4# composition is with to contrast 1# composition score suitable, and 2# composition score is the highest, apparently higher than control group and other groups.Relative to 1#, 3# and 4# composition, add the cigarette of 2# composition, its cigarette flavor harmony, the natural flavor of improvement and promoting or transferring cigarette perfume (or spice), increases pungent note, make cigarette flavor abundanter, increase the solid sense of fragrance, promote the mellow and full property of cigarette flavor, person experiences naturally easily to bring cigarette smoking, assorted gas, stimulation reduce, and overall sucking quality is improved.
Embodiment 3:
According to the formula in table 5, each component in table 5 except 70% ethanol is mixed, prepare the camellia extract composition with pungent fragrant note.Wherein 1# composition in contrast, only containing a kind of component Tea Flower medicinal extract.
Table 5
Embodiment 3 is prepared the camellia extract composition with pungent note that obtains according to the ratio in upper table 5, add 70% ethanol water, obtain camellia extract composition ethanolic solution.The camellia extract composition ethanolic solution with pungent note obtained evenly is sprayed onto on pipe tobacco by 0.025% of pipe tobacco weight, after baking, rolls into cigarette.Wherein 0# is as blank, on pipe tobacco, only spray the ethanol water of 70%.Then carry out sensory evaluating smoking's experiment by GB5606.4-2005, comparison scoring event of smokeing panel test is in table 6.
Table 6 Sensory Quality of Cigarette inspection original record
Smoking result shows: the score of 3# and 4# composition is with to contrast 1# composition score suitable, and 2# composition score is the highest, apparently higher than control group and other groups.Relative to 1#, 3# and 4# composition, add the cigarette of 2# composition, its cigarette flavor harmony, increase happy tobacco aroma, promote cigarette nature cigarette fragrant, increase pungent note, the rich of cigarette flavor is improved, increase the comfortableness of cigarette flavor, assorted gas, stimulation reduce, and overall sucking quality is improved.
Embodiment 4:
According to the formula in table 7, each component in table 7 except 70% ethanol is mixed, prepare the camellia extract composition with pungent fragrant note.Wherein 1# composition in contrast, only containing a kind of component Tea Flower medicinal extract.
Table 7
Embodiment 4 is prepared the camellia extract composition with pungent note that obtains according to the ratio in upper table 7, add 70% ethanol water, obtain camellia extract composition ethanolic solution.The camellia extract composition ethanolic solution with pungent note obtained evenly is sprayed onto on pipe tobacco by 0.045% of pipe tobacco weight, after baking, rolls into cigarette.Wherein 0# is as blank, on pipe tobacco, only spray the ethanol water of 70%.Then carry out sensory evaluating smoking's experiment by GB5606.4-2005, comparison scoring event of smokeing panel test is in table 8.
Table 8 Sensory Quality of Cigarette inspection original record
Smoking result shows: the score of 3# and 4# composition is with to contrast 1# composition score suitable, and 2# composition score is the highest, apparently higher than control group and other groups.Relative to 1#, 3# and 4# composition, add the cigarette of 2# composition, its cigarette flavor is coordinated, and fragrance is gentle and fragrance remaining time is long, increase pungent note, fragrance is mellow and full soft, improves alcohol and the degree of cigarette flavor, increases fragrance rich, set off nature cigarette fragrant, abirritate, improves mouthfeel.
Claims (114)
1. a camellia extract composition, formed by tea flower extract and pungent fragrant flavor confect, wherein said pungent spices is that clove bud oil, ennel oil, coriander extract, β-China pink are rare, eugenol and extract of cinnamomum cassia bark, wherein said tea flower extract is Tea Flower medicinal extract, wherein the content of each component is with parts by weight, is respectively:
Tea Flower medicinal extract 10-30;
Clove bud oil 0.05-0.15;
Ennel oil 0.1-0.2;
Coriander extract 0.02-0.08;
The rare 0.05-0.15 of β-China pink;
Eugenol 0.1-0.3;
Extract of cinnamomum cassia bark 0.2-0.3.
2. the combination of claim 1, wherein the weight portion of Tea Flower medicinal extract is 15-25.
3. the combination of claim 1, wherein the weight portion of Tea Flower medicinal extract is 18-22.
4. the combination of claim 1, wherein the weight portion of Tea Flower medicinal extract is 20.
5. the combination of claim 1, wherein the weight portion of clove bud oil is 0.08-0.12.
6. the combination of claim 1, wherein the weight portion of clove bud oil is 0.09-0.11.
7. the combination of claim 1, wherein the weight portion of clove bud oil is 0.1.
8. the combination of claim 1, wherein the weight portion of ennel oil is 0.12-0.18.
9. the combination of claim 1, wherein the weight portion of ennel oil is 0.13-0.16.
10. the combination of claim 1, wherein the weight portion of ennel oil is 0.15.
The combination of 11. claims 1, wherein the weight portion of coriander extract is 0.03-0.07.
The combination of 12. claims 1, wherein the weight portion of coriander extract is 0.04-0.06.
The combination of 13. claims 1, wherein the weight portion of coriander extract is 0.05.
The combination of 14. claims 1, the weight portion that wherein β-China pink is rare is 0.08-0.12.
The combination of 15. claims 1, the weight portion that wherein β-China pink is rare is 0.09-0.11.
The combination of 16. claims 1, the weight portion that wherein β-China pink is rare is 0.1.
The combination of 17. claims 1, wherein the weight portion of eugenol is 0.15-0.25.
The combination of 18. claims 1, wherein the weight portion of eugenol is 0.18-0.22.
The combination of 19. claims 1, wherein the weight portion of eugenol is 0.2.
The combination of 20. claims 1, wherein the weight portion of extract of cinnamomum cassia bark is 0.22-0.28.
The combination of 21. claims 1, wherein the weight portion of extract of cinnamomum cassia bark is 0.24-0.26.
The combination of 22. claims 1, wherein the weight portion of extract of cinnamomum cassia bark is 0.25.
23. 1 kinds of camellia extract composition, formed by tea flower extract and pungent fragrant flavor confect, wherein said pungent spices is carrot seed oil, aniseed oil, ginger oil, sage clary oil, radix valerianae extract, extract of cinnamomum cassia bark, radix tarxaci extract, wherein said tea flower extract is essential oil of the flower of Camellia sinensis, wherein the content of each component is with parts by weight, is respectively:
Essential oil of the flower of Camellia sinensis 5-15;
Carrot seed oil 0.1-0.2;
Aniseed oil 0.05-0.15;
Ginger oil 0.02-0.08;
Sage clary oil 0.05-0.15;
Radix valerianae extract 0.2-0.8;
Extract of cinnamomum cassia bark 0.2-0.3;
Radix tarxaci extract 0.1-0.2.
The composition of 24. claims 23, wherein the weight portion of essential oil of the flower of Camellia sinensis is 8-12.
The composition of 25. claims 23, wherein the weight portion of essential oil of the flower of Camellia sinensis is 9-11.
The composition of 26. claims 23, wherein the weight portion of essential oil of the flower of Camellia sinensis is 10.
The composition of 27. claims 23, wherein the weight portion of carrot seed oil is 0.12-0.18.
The composition of 28. claims 23, wherein the weight portion of carrot seed oil is 0.13-0.16.
The composition of 29. claims 23, wherein the weight portion of carrot seed oil is 0.15.
The composition of 30. claims 23, wherein the weight portion of aniseed oil is 0.08-0.12.
The composition of 31. claims 23, wherein the weight portion of aniseed oil is 0.09-0.11.
The composition of 32. claims 23, wherein the weight portion of aniseed oil is 0.1.
The composition of 33. claims 23, wherein the weight portion of ginger oil is 0.03-0.07.
The composition of 34. claims 23, wherein the weight portion of ginger oil is 0.04-0.06.
The composition of 35. claims 23, wherein the weight portion of ginger oil is 0.05.
The composition of 36. claims 23, wherein the weight portion of sage clary oil is 0.08-0.12.
The composition of 37. claims 23, wherein the weight portion of sage clary oil is 0.09-0.11.
The composition of 38. claims 23, wherein the weight portion of sage clary oil is 0.1.
The composition of 39. claims 23, wherein the weight portion of radix valerianae extract is 0.3-0.7.
The composition of 40. claims 23, wherein the weight portion of radix valerianae extract is 0.4-0.6.
The composition of 41. claims 23, wherein the weight portion of radix valerianae extract is 0.55.
The composition of 42. claims 23, wherein the weight portion of extract of cinnamomum cassia bark is 0.22-0.28.
The composition of 43. claims 23, wherein the weight portion of extract of cinnamomum cassia bark is 0.24-0.26.
The composition of 44. claims 23, wherein the weight portion of extract of cinnamomum cassia bark is 0.25.
The composition of 45. claims 23, wherein the weight portion of radix tarxaci extract is 0.12-0.18.
The composition of 46. claims 23, wherein the weight portion of radix tarxaci extract is 0.13-0.16.
The composition of 47. claims 23, wherein the weight portion of radix tarxaci extract is 0.15.
48. 1 kinds of camellia extract composition, formed by tea flower extract and pungent fragrant flavor confect, wherein said pungent spices is that carrot seed oil, aniseed oil, ginger oil, β-China pink are rare, radix valerianae extract, extract of cinnamomum cassia bark, radix tarxaci extract, wherein said tea flower extract is Tea Flower absolute oil, wherein the content of each component is with parts by weight, is respectively: Tea Flower absolute oil 15-35;
Carrot seed oil 0.1-0.2;
Aniseed oil 0.05-0.15;
Ginger oil 0.02-0.08;
The rare 0.1-0.2 of β-China pink;
Radix valerianae extract 0.2-0.8;
Extract of cinnamomum cassia bark 0.2-0.3;
Radix tarxaci extract 0.1-0.2.
The composition of 49. claims 48, wherein the weight portion of Tea Flower absolute oil is 20-30.
The composition of 50. claims 48, wherein the weight portion of Tea Flower absolute oil is 22-28.
The composition of 51. claims 48, wherein the weight portion of Tea Flower absolute oil is 25.
The composition of 52. claims 48, wherein the weight portion of carrot seed oil is 0.12-0.18.
The composition of 53. claims 48, wherein the weight portion of carrot seed oil is 0.13-0.16.
The composition of 54. claims 48, wherein the weight portion of carrot seed oil is 0.15.
The composition of 55. claims 48, wherein the weight portion of aniseed oil is 0.08-0.12.
The composition of 56. claims 48, wherein the weight portion of aniseed oil is 0.09-0.11.
The composition of 57. claims 48, wherein the weight portion of aniseed oil is 0.1.
The composition of 58. claims 48, wherein the weight portion of ginger oil is 0.03-0.07.
The composition of 59. claims 48, wherein the weight portion of ginger oil is 0.04-0.06.
The composition of 60. claims 48, wherein the weight portion of ginger oil is 0.05.
The composition of 61. claims 48, the weight portion that wherein β-China pink is rare is 0.12-0.18.
The composition of 62. claims 48, the weight portion that wherein β-China pink is rare is 0.13-0.16.
The composition of 63. claims 48, the weight portion that wherein β-China pink is rare is 0.15.
The composition of 64. claims 48, wherein the weight portion of radix valerianae extract is 0.3-0.7.
The composition of 65. claims 48, wherein the weight portion of radix valerianae extract is 0.4-0.6.
The composition of 66. claims 48, wherein the weight portion of radix valerianae extract is 0.55.
The composition of 67. claims 48, wherein the weight portion of extract of cinnamomum cassia bark is 0.22-0.28.
The composition of 68. claims 48, wherein the weight portion of extract of cinnamomum cassia bark is 0.24-0.26.
The composition of 69. claims 48, wherein the weight portion of extract of cinnamomum cassia bark is 0.25.
The composition of 70. claims 48, wherein the weight portion of radix tarxaci extract is 0.12-0.18.
The composition of 71. claims 48, wherein the weight portion of radix tarxaci extract is 0.13-0.16.
The composition of 72. claims 48, wherein the weight portion of radix tarxaci extract is 0.15.
73. 1 kinds of camellia extract composition, formed by tea flower extract and pungent fragrant flavor confect, wherein said pungent spices is that clove bud oil, aniseed oil, ennel oil, β-China pink are rare, sage clary oil, extract of cinnamomum cassia bark, radix tarxaci extract, wherein said tea flower extract is Tea Flower tincture, wherein the content of each component is with parts by weight, is respectively: Tea Flower tincture 20-40;
Clove bud oil 0.02-0.08;
Aniseed oil 0.05-0.15;
Ennel oil 0.02-0.08;
The rare 0.1-0.2 of β-China pink;
Sage clary oil 0.05-0.15;
Extract of cinnamomum cassia bark 0.1-0.2;
Radix tarxaci extract 0.2-0.3.
The composition of 74. claims 73, wherein the weight portion of Tea Flower tincture is 25-35.
The composition of 75. claims 73, wherein the weight portion of Tea Flower tincture is 28-32.
The composition of 76. claims 73, wherein the weight portion of Tea Flower tincture is 30.
The composition of 77. claims 73, wherein the weight portion of clove bud oil is 0.03-0.07.
The composition of 78. claims 73, wherein the weight portion of clove bud oil is 0.04-0.06.
The composition of 79. claims 73, wherein the weight portion of clove bud oil is 0.05.
The composition of 80. claims 73, wherein the weight portion of aniseed oil is 0.08-0.12.
The composition of 81. claims 73, wherein the weight portion of aniseed oil is 0.09-0.11.
The composition of 82. claims 73, wherein the weight portion of aniseed oil is 0.1.
The composition of 83. claims 73, wherein the weight portion of ennel oil is 0.03-0.07.
The composition of 84. claims 73, wherein the weight portion of ennel oil is 0.04-0.06.
The composition of 85. claims 73, wherein the weight portion of ennel oil is 0.05.
The composition of 86. claims 73, the weight portion that wherein β-China pink is rare is 0.12-0.18.
The composition of 87. claims 73, the weight portion that wherein β-China pink is rare is 0.13-0.16.
The composition of 88. claims 73, the weight portion that wherein β-China pink is rare is 0.15.
The composition of 89. claims 73, wherein the weight portion of sage clary oil is 0.08-0.12.
The composition of 90. claims 73, wherein the weight portion of sage clary oil is 0.09-0.11.
The composition of 91. claims 73, wherein the weight portion of sage clary oil is 0.1.
The composition of 92. claims 73, wherein the weight portion of extract of cinnamomum cassia bark is 0.12-0.18.
The composition of 93. claims 73, wherein the weight portion of extract of cinnamomum cassia bark is 0.13-0.16.
The composition of 94. claims 73, wherein the weight portion of extract of cinnamomum cassia bark is 0.15.
The composition of 95. claims 73, wherein the weight portion of radix tarxaci extract is 0.22-0.28.
The composition of 96. claims 73, wherein the weight portion of radix tarxaci extract is 0.24-0.26.
The composition of 97. claims 73, wherein the weight portion of radix tarxaci extract is 0.25.
The composition of 98. any one of claim 1 to 97, also comprises ethanol in said composition.
The composition of 99. claims 98, wherein said ethanol is the ethanol water of 50 ~ 95%.
The composition of 100. claims 98, wherein said ethanol is the ethanol water of 60 ~ 80%.
The composition of 101. claims 98, wherein said ethanol is the ethanol water of 65 ~ 75%.
The composition of 102. claims 98, wherein said ethanol is the ethanol water of 70%.
103. any one of claim 99 to 102 composition, wherein the weight portion content of ethanol water is 60-90.
104. any one of claim 99 to 102 composition, wherein the weight portion content of ethanol water is 75-80.
105. any one of claim 99 to 102 composition, wherein the weight portion content of ethanol water is 85-90.
106. any one of claim 99 to 102 composition, wherein the weight portion content of ethanol water is 70-75.
107. any one of claim 99 to 102 composition, wherein the weight portion content of ethanol water is 65-70.
The purposes of composition in cigarette of 108. any one of claim 1 to 107.
The composition of 109. any one of claim 1 to 107 is as the purposes of cigarette additive.
The composition of 110. any one of claim 1 to 107 is as the purposes of cigarette flavors.
The purposes of 111. claims 110, said composition is used for pipe tobacco, thin slice, the internal lining paper of cigarette, filter stick as cigarette flavors.
112. one kinds of cigarette, it comprises the composition of any one of claim 1 to 107.
The cigarette of 113. claims 112, described composition is the composition containing ethanol water.
The cigarette of 114. claims 112, the consumption of the described composition containing ethanol water is 0.005 ~ 0.05% of pipe tobacco weight.
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