CN103227339A - 产生可再生氢并截留二氧化碳的电化学系统、装置和方法 - Google Patents
产生可再生氢并截留二氧化碳的电化学系统、装置和方法 Download PDFInfo
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- CN103227339A CN103227339A CN2013101087737A CN201310108773A CN103227339A CN 103227339 A CN103227339 A CN 103227339A CN 2013101087737 A CN2013101087737 A CN 2013101087737A CN 201310108773 A CN201310108773 A CN 201310108773A CN 103227339 A CN103227339 A CN 103227339A
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- Prior art keywords
- carbon dioxide
- hydrogen
- acid
- alkali
- carbonate
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
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- CURLTUGMZLYLDI-UHFFFAOYSA-N Carbon dioxide Chemical compound O=C=O CURLTUGMZLYLDI-UHFFFAOYSA-N 0.000 title claims abstract description 703
- 229910002092 carbon dioxide Inorganic materials 0.000 title claims abstract description 351
- 239000001569 carbon dioxide Substances 0.000 title claims abstract description 350
- 239000001257 hydrogen Substances 0.000 title claims abstract description 199
- 229910052739 hydrogen Inorganic materials 0.000 title claims abstract description 199
- UFHFLCQGNIYNRP-UHFFFAOYSA-N Hydrogen Chemical compound [H][H] UFHFLCQGNIYNRP-UHFFFAOYSA-N 0.000 title claims abstract description 179
- 238000004519 manufacturing process Methods 0.000 title abstract description 17
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 claims abstract description 206
- 239000002253 acid Substances 0.000 claims abstract description 140
- 239000003792 electrolyte Substances 0.000 claims abstract description 121
- 238000005868 electrolysis reaction Methods 0.000 claims description 219
- 238000000034 method Methods 0.000 claims description 161
- 239000003513 alkali Substances 0.000 claims description 151
- BVKZGUZCCUSVTD-UHFFFAOYSA-L Carbonate Chemical compound [O-]C([O-])=O BVKZGUZCCUSVTD-UHFFFAOYSA-L 0.000 claims description 119
- 239000000243 solution Substances 0.000 claims description 105
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 claims description 103
- 239000001301 oxygen Substances 0.000 claims description 103
- 229910052760 oxygen Inorganic materials 0.000 claims description 103
- BVKZGUZCCUSVTD-UHFFFAOYSA-M Bicarbonate Chemical compound OC([O-])=O BVKZGUZCCUSVTD-UHFFFAOYSA-M 0.000 claims description 85
- 239000008151 electrolyte solution Substances 0.000 claims description 81
- 239000000047 product Substances 0.000 claims description 72
- 238000006243 chemical reaction Methods 0.000 claims description 64
- OKKJLVBELUTLKV-UHFFFAOYSA-N Methanol Chemical compound OC OKKJLVBELUTLKV-UHFFFAOYSA-N 0.000 claims description 57
- XSQUKJJJFZCRTK-UHFFFAOYSA-N Urea Chemical compound NC(N)=O XSQUKJJJFZCRTK-UHFFFAOYSA-N 0.000 claims description 41
- BDAGIHXWWSANSR-UHFFFAOYSA-N methanoic acid Natural products OC=O BDAGIHXWWSANSR-UHFFFAOYSA-N 0.000 claims description 40
- 239000000203 mixture Substances 0.000 claims description 27
- 239000000463 material Substances 0.000 claims description 26
- UGFAIRIUMAVXCW-UHFFFAOYSA-N Carbon monoxide Chemical compound [O+]#[C-] UGFAIRIUMAVXCW-UHFFFAOYSA-N 0.000 claims description 25
- VTYYLEPIZMXCLO-UHFFFAOYSA-L Calcium carbonate Chemical compound [Ca+2].[O-]C([O-])=O VTYYLEPIZMXCLO-UHFFFAOYSA-L 0.000 claims description 24
- 229910002091 carbon monoxide Inorganic materials 0.000 claims description 24
- GPRLSGONYQIRFK-UHFFFAOYSA-N hydron Chemical compound [H+] GPRLSGONYQIRFK-UHFFFAOYSA-N 0.000 claims description 22
- VEXZGXHMUGYJMC-UHFFFAOYSA-M Chloride anion Chemical compound [Cl-] VEXZGXHMUGYJMC-UHFFFAOYSA-M 0.000 claims description 21
- 239000004202 carbamide Substances 0.000 claims description 21
- OSWFIVFLDKOXQC-UHFFFAOYSA-N 4-(3-methoxyphenyl)aniline Chemical compound COC1=CC=CC(C=2C=CC(N)=CC=2)=C1 OSWFIVFLDKOXQC-UHFFFAOYSA-N 0.000 claims description 20
- 235000019253 formic acid Nutrition 0.000 claims description 20
- 239000004033 plastic Substances 0.000 claims description 16
- 229920003023 plastic Polymers 0.000 claims description 16
- 238000001556 precipitation Methods 0.000 claims description 16
- ZAMOUSCENKQFHK-UHFFFAOYSA-N Chlorine atom Chemical compound [Cl] ZAMOUSCENKQFHK-UHFFFAOYSA-N 0.000 claims description 15
- 238000003860 storage Methods 0.000 claims description 15
- IJGRMHOSHXDMSA-UHFFFAOYSA-N Atomic nitrogen Chemical compound N#N IJGRMHOSHXDMSA-UHFFFAOYSA-N 0.000 claims description 14
- PMZURENOXWZQFD-UHFFFAOYSA-L Sodium Sulfate Chemical compound [Na+].[Na+].[O-]S([O-])(=O)=O PMZURENOXWZQFD-UHFFFAOYSA-L 0.000 claims description 14
- 239000000460 chlorine Substances 0.000 claims description 14
- 229910052801 chlorine Inorganic materials 0.000 claims description 14
- 230000008859 change Effects 0.000 claims description 13
- -1 proton Chemical compound 0.000 claims description 13
- 239000007787 solid Substances 0.000 claims description 13
- 229910000019 calcium carbonate Inorganic materials 0.000 claims description 12
- 239000004035 construction material Substances 0.000 claims description 10
- 229910052500 inorganic mineral Inorganic materials 0.000 claims description 10
- 239000011707 mineral Substances 0.000 claims description 10
- 238000002360 preparation method Methods 0.000 claims description 9
- TZIHFWKZFHZASV-UHFFFAOYSA-N methyl formate Chemical compound COC=O TZIHFWKZFHZASV-UHFFFAOYSA-N 0.000 claims description 8
- BHPQYMZQTOCNFJ-UHFFFAOYSA-N Calcium cation Chemical compound [Ca+2] BHPQYMZQTOCNFJ-UHFFFAOYSA-N 0.000 claims description 7
- 239000010425 asbestos Substances 0.000 claims description 7
- 229910001424 calcium ion Inorganic materials 0.000 claims description 7
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- 239000011347 resin Substances 0.000 claims description 7
- 229920005989 resin Polymers 0.000 claims description 7
- 229910052895 riebeckite Inorganic materials 0.000 claims description 7
- 229910052938 sodium sulfate Inorganic materials 0.000 claims description 7
- 235000011152 sodium sulphate Nutrition 0.000 claims description 7
- 238000011282 treatment Methods 0.000 claims description 7
- WYTGDNHDOZPMIW-RCBQFDQVSA-N alstonine Natural products C1=CC2=C3C=CC=CC3=NC2=C2N1C[C@H]1[C@H](C)OC=C(C(=O)OC)[C@H]1C2 WYTGDNHDOZPMIW-RCBQFDQVSA-N 0.000 claims description 6
- 239000003054 catalyst Substances 0.000 claims description 5
- 238000005065 mining Methods 0.000 claims description 5
- QGZKDVFQNNGYKY-UHFFFAOYSA-N Ammonia Chemical compound N QGZKDVFQNNGYKY-UHFFFAOYSA-N 0.000 claims description 4
- 239000004927 clay Substances 0.000 claims description 4
- 239000000454 talc Substances 0.000 claims description 4
- 229910052623 talc Inorganic materials 0.000 claims description 4
- 235000012222 talc Nutrition 0.000 claims description 4
- 239000000853 adhesive Substances 0.000 claims description 3
- 230000001070 adhesive effect Effects 0.000 claims description 3
- 239000002969 artificial stone Substances 0.000 claims description 3
- 239000006227 byproduct Substances 0.000 claims description 3
- FYHXNYLLNIKZMR-UHFFFAOYSA-N calcium;carbonic acid Chemical compound [Ca].OC(O)=O FYHXNYLLNIKZMR-UHFFFAOYSA-N 0.000 claims description 3
- 239000011440 grout Substances 0.000 claims description 3
- 239000004568 cement Substances 0.000 claims description 2
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- 238000007600 charging Methods 0.000 claims description 2
- 239000012153 distilled water Substances 0.000 claims description 2
- 239000010440 gypsum Substances 0.000 claims description 2
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- 230000007062 hydrolysis Effects 0.000 claims description 2
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- 239000011505 plaster Substances 0.000 claims description 2
- 230000001105 regulatory effect Effects 0.000 claims 1
- 239000007789 gas Substances 0.000 abstract description 75
- 239000002585 base Substances 0.000 abstract description 59
- 239000000446 fuel Substances 0.000 abstract description 31
- MYMOFIZGZYHOMD-UHFFFAOYSA-N Dioxygen Chemical compound O=O MYMOFIZGZYHOMD-UHFFFAOYSA-N 0.000 abstract 1
- 229910001882 dioxygen Inorganic materials 0.000 abstract 1
- 230000001172 regenerating effect Effects 0.000 description 39
- 239000012298 atmosphere Substances 0.000 description 38
- 239000012528 membrane Substances 0.000 description 32
- HEMHJVSKTPXQMS-UHFFFAOYSA-M Sodium hydroxide Chemical compound [OH-].[Na+] HEMHJVSKTPXQMS-UHFFFAOYSA-M 0.000 description 31
- XLYOFNOQVPJJNP-UHFFFAOYSA-M hydroxide Chemical compound [OH-] XLYOFNOQVPJJNP-UHFFFAOYSA-M 0.000 description 30
- 230000008569 process Effects 0.000 description 28
- 150000007516 brønsted-lowry acids Chemical class 0.000 description 27
- 150000007528 brønsted-lowry bases Chemical class 0.000 description 27
- 238000000926 separation method Methods 0.000 description 27
- 150000002431 hydrogen Chemical class 0.000 description 24
- 150000002500 ions Chemical class 0.000 description 24
- 235000002639 sodium chloride Nutrition 0.000 description 21
- 239000012141 concentrate Substances 0.000 description 20
- 239000000126 substance Substances 0.000 description 20
- CSCPPACGZOOCGX-UHFFFAOYSA-N Acetone Chemical compound CC(C)=O CSCPPACGZOOCGX-UHFFFAOYSA-N 0.000 description 18
- VNWKTOKETHGBQD-UHFFFAOYSA-N methane Chemical compound C VNWKTOKETHGBQD-UHFFFAOYSA-N 0.000 description 18
- 150000001450 anions Chemical class 0.000 description 17
- 230000004888 barrier function Effects 0.000 description 17
- 150000001768 cations Chemical class 0.000 description 17
- CDBYLPFSWZWCQE-UHFFFAOYSA-L Sodium Carbonate Chemical compound [Na+].[Na+].[O-]C([O-])=O CDBYLPFSWZWCQE-UHFFFAOYSA-L 0.000 description 16
- LFQSCWFLJHTTHZ-UHFFFAOYSA-N Ethanol Chemical compound CCO LFQSCWFLJHTTHZ-UHFFFAOYSA-N 0.000 description 15
- LYCAIKOWRPUZTN-UHFFFAOYSA-N Ethylene glycol Chemical compound OCCO LYCAIKOWRPUZTN-UHFFFAOYSA-N 0.000 description 15
- 238000010586 diagram Methods 0.000 description 15
- ODINCKMPIJJUCX-UHFFFAOYSA-N Calcium oxide Chemical compound [Ca]=O ODINCKMPIJJUCX-UHFFFAOYSA-N 0.000 description 14
- KWYUFKZDYYNOTN-UHFFFAOYSA-M Potassium hydroxide Chemical compound [OH-].[K+] KWYUFKZDYYNOTN-UHFFFAOYSA-M 0.000 description 14
- QAOWNCQODCNURD-UHFFFAOYSA-N Sulfuric acid Chemical compound OS(O)(=O)=O QAOWNCQODCNURD-UHFFFAOYSA-N 0.000 description 14
- 230000005611 electricity Effects 0.000 description 14
- 238000002848 electrochemical method Methods 0.000 description 13
- 239000012267 brine Substances 0.000 description 12
- BVKZGUZCCUSVTD-UHFFFAOYSA-N carbonic acid Chemical compound OC(O)=O BVKZGUZCCUSVTD-UHFFFAOYSA-N 0.000 description 12
- 239000007788 liquid Substances 0.000 description 12
- HPALAKNZSZLMCH-UHFFFAOYSA-M sodium;chloride;hydrate Chemical compound O.[Na+].[Cl-] HPALAKNZSZLMCH-UHFFFAOYSA-M 0.000 description 12
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 description 11
- 230000015572 biosynthetic process Effects 0.000 description 11
- 229910052799 carbon Inorganic materials 0.000 description 11
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- 235000008733 Citrus aurantifolia Nutrition 0.000 description 10
- ZHNUHDYFZUAESO-UHFFFAOYSA-N Formamide Chemical compound NC=O ZHNUHDYFZUAESO-UHFFFAOYSA-N 0.000 description 10
- 235000011941 Tilia x europaea Nutrition 0.000 description 10
- 239000010408 film Substances 0.000 description 10
- 239000012530 fluid Substances 0.000 description 10
- 239000004571 lime Substances 0.000 description 10
- PXHVJJICTQNCMI-UHFFFAOYSA-N Nickel Chemical compound [Ni] PXHVJJICTQNCMI-UHFFFAOYSA-N 0.000 description 9
- 238000005516 engineering process Methods 0.000 description 9
- 235000010755 mineral Nutrition 0.000 description 9
- 150000003839 salts Chemical class 0.000 description 9
- CSNNHWWHGAXBCP-UHFFFAOYSA-L Magnesium sulfate Chemical compound [Mg+2].[O-][S+2]([O-])([O-])[O-] CSNNHWWHGAXBCP-UHFFFAOYSA-L 0.000 description 8
- UIIMBOGNXHQVGW-UHFFFAOYSA-M Sodium bicarbonate Chemical compound [Na+].OC([O-])=O UIIMBOGNXHQVGW-UHFFFAOYSA-M 0.000 description 8
- 238000013461 design Methods 0.000 description 8
- 230000007935 neutral effect Effects 0.000 description 8
- BASFCYQUMIYNBI-UHFFFAOYSA-N platinum Chemical compound [Pt] BASFCYQUMIYNBI-UHFFFAOYSA-N 0.000 description 8
- 238000012545 processing Methods 0.000 description 8
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- QTBSBXVTEAMEQO-UHFFFAOYSA-M Acetate Chemical compound CC([O-])=O QTBSBXVTEAMEQO-UHFFFAOYSA-M 0.000 description 6
- 239000002551 biofuel Substances 0.000 description 6
- 150000001875 compounds Chemical class 0.000 description 6
- ZLNQQNXFFQJAID-UHFFFAOYSA-L magnesium carbonate Chemical class [Mg+2].[O-]C([O-])=O ZLNQQNXFFQJAID-UHFFFAOYSA-L 0.000 description 6
- 229920000642 polymer Polymers 0.000 description 6
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- IKHGUXGNUITLKF-XPULMUKRSA-N acetaldehyde Chemical compound [14CH]([14CH3])=O IKHGUXGNUITLKF-XPULMUKRSA-N 0.000 description 5
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- 229910000021 magnesium carbonate Inorganic materials 0.000 description 5
- WSFSSNUMVMOOMR-NJFSPNSNSA-N methanone Chemical compound O=[14CH2] WSFSSNUMVMOOMR-NJFSPNSNSA-N 0.000 description 5
- 229910000029 sodium carbonate Inorganic materials 0.000 description 5
- NWUYHJFMYQTDRP-UHFFFAOYSA-N 1,2-bis(ethenyl)benzene;1-ethenyl-2-ethylbenzene;styrene Chemical compound C=CC1=CC=CC=C1.CCC1=CC=CC=C1C=C.C=CC1=CC=CC=C1C=C NWUYHJFMYQTDRP-UHFFFAOYSA-N 0.000 description 4
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- FAPWRFPIFSIZLT-UHFFFAOYSA-M Sodium chloride Chemical compound [Na+].[Cl-] FAPWRFPIFSIZLT-UHFFFAOYSA-M 0.000 description 4
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- H01M8/0606—Combination of fuel cells with means for production of reactants or for treatment of residues with means for production of gaseous reactants
- H01M8/0656—Combination of fuel cells with means for production of reactants or for treatment of residues with means for production of gaseous reactants by electrochemical means
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- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
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- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
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Abstract
Description
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CN110914478A (zh) * | 2017-07-18 | 2020-03-24 | 西门子股份公司 | Co2电解槽 |
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CN113316482B (zh) * | 2019-01-22 | 2023-08-25 | 东京瓦斯株式会社 | 反应装置以及燃料电池发电系统 |
CN113144904A (zh) * | 2020-01-23 | 2021-07-23 | 住友重机械工业株式会社 | 氢回收装置、氢回收方法及二氧化碳固定系统 |
CN113144904B (zh) * | 2020-01-23 | 2023-06-30 | 住友重机械工业株式会社 | 氢回收装置、氢回收方法及二氧化碳固定系统 |
WO2023087370A1 (zh) * | 2021-11-17 | 2023-05-25 | 国家电投集团科学技术研究院有限公司 | 耦合分级电解/热解制氢的二氧化碳捕集方法 |
WO2024016114A1 (zh) * | 2022-07-18 | 2024-01-25 | 势加透博(北京)科技有限公司 | 碳捕集耦合制氢的方法及装置 |
Also Published As
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US20080245672A1 (en) | 2008-10-09 |
CN103227339B (zh) | 2016-03-09 |
CA2682952C (en) | 2016-06-14 |
EP2132820A4 (en) | 2014-12-24 |
AU2008237264B2 (en) | 2012-09-20 |
US20080245660A1 (en) | 2008-10-09 |
CN101981744A (zh) | 2011-02-23 |
WO2008124538A1 (en) | 2008-10-16 |
CA2682952A1 (en) | 2008-10-16 |
EP2132820A1 (en) | 2009-12-16 |
AU2008237264A1 (en) | 2008-10-16 |
US8227127B2 (en) | 2012-07-24 |
US20080248350A1 (en) | 2008-10-09 |
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