CA2253987A1 - Method of manufacturing fuel cells and fuel cells manufactured by the method - Google Patents

Method of manufacturing fuel cells and fuel cells manufactured by the method

Info

Publication number
CA2253987A1
CA2253987A1 CA002253987A CA2253987A CA2253987A1 CA 2253987 A1 CA2253987 A1 CA 2253987A1 CA 002253987 A CA002253987 A CA 002253987A CA 2253987 A CA2253987 A CA 2253987A CA 2253987 A1 CA2253987 A1 CA 2253987A1
Authority
CA
Canada
Prior art keywords
adhesive
polymer electrolyte
electrolyte film
separators
fuel cells
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Granted
Application number
CA002253987A
Other languages
French (fr)
Other versions
CA2253987C (en
Inventor
Seiji Mizuno
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Toyota Motor Corp
Original Assignee
Toyota Motor Corp
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Toyota Motor Corp filed Critical Toyota Motor Corp
Publication of CA2253987A1 publication Critical patent/CA2253987A1/en
Application granted granted Critical
Publication of CA2253987C publication Critical patent/CA2253987C/en
Anticipated expiration legal-status Critical
Expired - Fee Related legal-status Critical Current

Links

Classifications

    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0271Sealing or supporting means around electrodes, matrices or membranes
    • H01M8/028Sealing means characterised by their material
    • H01M8/0284Organic resins; Organic polymers
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0271Sealing or supporting means around electrodes, matrices or membranes
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1004Fuel cells with solid electrolytes characterised by membrane-electrode assemblies [MEA]
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M2008/1095Fuel cells with polymeric electrolytes
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30Hydrogen technology
    • Y02E60/50Fuel cells
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02PCLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50Manufacturing or production processes characterised by the final manufactured product
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10TTECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
    • Y10T29/00Metal working
    • Y10T29/49Method of mechanical manufacture
    • Y10T29/49002Electrical device making
    • Y10T29/49108Electric battery cell making
    • Y10T29/49114Electric battery cell making including adhesively bonding

Abstract

The method of the present invention enhances the adhesive strength of a polymer electrolyte film via an adhesive and thereby manufactures a fuel cell having the high reliability for the gas sealing property. The method exposes a joint body, which has been prepared by interposing a polymer electrolyte film between an anode and a cathode and bonding them, to an atmosphere having a temperature of 25°C and a humidity of 50%
over one hour (S110). The method then provides a pair of separators and applies an adhesive on specific areas of the separators, which are directly joined with the polymer electrolyte film (S120). The adhesive used here is a modified rubber adhesive that is a mixture of epoxy resin and modified silicone and has a modulus of elasticity of not greater than 10 MPa and a durometer A hardness of not greater than 90 after cure. The method subsequently lays the pair of separators upon the joint body and cures the adhesive for bonding the separators directly to the polymer electrolyte film (S130 and S140). The process of step S110 causes the polymer electrolyte film to have a water content ~ of not greater than 4. This effectively ensures the sufficient adhesive strength of the polymer electrolyte film via the adhesive.
CA002253987A 1997-11-21 1998-11-12 Method of manufacturing fuel cells and fuel cells manufactured by the method Expired - Fee Related CA2253987C (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP33812197A JP3918265B2 (en) 1997-11-21 1997-11-21 Manufacturing method of fuel cell
JP9-338121 1997-11-21

Publications (2)

Publication Number Publication Date
CA2253987A1 true CA2253987A1 (en) 1999-05-21
CA2253987C CA2253987C (en) 2003-04-01

Family

ID=18315119

Family Applications (1)

Application Number Title Priority Date Filing Date
CA002253987A Expired - Fee Related CA2253987C (en) 1997-11-21 1998-11-12 Method of manufacturing fuel cells and fuel cells manufactured by the method

Country Status (4)

Country Link
US (1) US6733916B2 (en)
EP (1) EP0918362A3 (en)
JP (1) JP3918265B2 (en)
CA (1) CA2253987C (en)

Families Citing this family (54)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE19829142A1 (en) * 1998-06-30 2000-01-05 Manhattan Scientifics Inc Gas-tight combination of bipolar plate and membrane-electrode assembly of polymer electrolyte membrane fuel cells
US6852440B1 (en) 1998-08-10 2005-02-08 Axiva Gmbh Fuel cell with improved long term performance, method for operating a PME fuel cell and PME fuel cell battery
EP1073138B1 (en) * 1999-07-26 2012-05-02 Tigers Polymer Corporation Sealing structure of fuel cell and process for molding rubber packing
DE19962682A1 (en) * 1999-12-23 2001-07-05 Siemens Ag Fuel cell stack, the use of a fuel cell stack and a method for assembling a fuel cell stack
JP2001236971A (en) * 2000-02-24 2001-08-31 Fuji Electric Co Ltd Method of producing solid high polymer fuel cell
JP3712592B2 (en) * 2000-05-02 2005-11-02 本田技研工業株式会社 Manufacturing method of fuel cell
JP3660205B2 (en) * 2000-05-02 2005-06-15 本田技研工業株式会社 Fuel cell and manufacturing method thereof
DE10121176B4 (en) 2000-05-02 2008-05-21 Honda Giken Kogyo K.K. A fuel cell having a sealant for sealing a solid polymer electrolyte membrane. A fuel cell stack and a process for producing the same
US7108936B2 (en) * 2000-05-08 2006-09-19 Honda Giken Kogyo Kabushiki Kaisha Fuel cell assembly
US6730426B2 (en) * 2001-01-12 2004-05-04 Mosaic Energy, Llc Integral sealing method for fuel cell separator plates
JP4043724B2 (en) * 2001-02-14 2008-02-06 本田技研工業株式会社 Unit fuel cell and fuel cell stack manufacturing method
JP4530122B2 (en) * 2001-03-09 2010-08-25 Nok株式会社 gasket
TW488111B (en) 2001-04-16 2002-05-21 Asia Pacific Fuel Cell Tech Anode stream recirculation system for a fuel cell
JP4000790B2 (en) 2001-06-08 2007-10-31 トヨタ自動車株式会社 Fuel cell having seal structure
JP4682453B2 (en) * 2001-06-08 2011-05-11 トヨタ自動車株式会社 Method and apparatus for applying solid component-containing liquid composition
JP3998438B2 (en) * 2001-06-22 2007-10-24 信越化学工業株式会社 Adhesive for polymer electrolyte fuel cells
JP4383008B2 (en) 2001-07-06 2009-12-16 本田技研工業株式会社 Fuel cell separator, method of laminating membrane / electrode assembly, and laminating apparatus
TW533620B (en) 2001-07-24 2003-05-21 Asia Pacific Fuel Cell Tech Metal hydride hydrogen storage canister design and its manufacture
TW511316B (en) 2001-08-15 2002-11-21 Asia Pacific Fuel Cell Tech Diaphragm pump and anode stream recirculation system using such pump for a fuel cell
CN1405915A (en) * 2001-08-16 2003-03-26 亚太燃料电池科技股份有限公司 Module element of proton exchange film fuel cell and moudule cell unit
DE60315153T2 (en) 2002-05-09 2008-04-10 Honda Giken Kogyo K.K. FUEL CELL ASSEMBLY AND METHOD FOR BINDING A DISCONNECTOR AND AN ELECTROLYTIC COATING OF A FUEL CELL ASSEMBLY GROUP
US7147959B2 (en) 2002-05-31 2006-12-12 Umicore Ag & Co. Kg Process for the manufacture of membrane-electrode-assemblies using catalyst-coated membranes
US7393369B2 (en) * 2002-06-11 2008-07-01 Trulite, Inc. Apparatus, system, and method for generating hydrogen
DE10250434A1 (en) * 2002-10-30 2004-05-13 Ab Skf Module for a fuel cell arrangement
US20040197629A1 (en) * 2003-01-20 2004-10-07 Yasuo Arishima Electric power generating element for fuel cell and fuel cell using the same
CN1536698B (en) 2003-04-02 2010-12-15 松下电器产业株式会社 Electrolyte film structure for fuel cell, MEA structure and fuel cell
US7556660B2 (en) 2003-06-11 2009-07-07 James Kevin Shurtleff Apparatus and system for promoting a substantially complete reaction of an anhydrous hydride reactant
TWI241046B (en) * 2003-12-12 2005-10-01 Asia Pacific Fuel Cell Tech Sealing structure of modulized proton-exchange-membrane fuel battery
JP4862243B2 (en) 2003-12-24 2012-01-25 トヨタ自動車株式会社 Fuel cell stack
JP2007533088A (en) * 2004-04-13 2007-11-15 ユミコア・アクチエンゲゼルシャフト・ウント・コムパニー・コマンディットゲゼルシャフト Multilayer electrode assembly (ML-MEA) and method of manufacturing the same
WO2005104287A1 (en) * 2004-04-26 2005-11-03 Toyota Jidosha Kabushiki Kaisha Fuel cell module
JP2006032041A (en) * 2004-07-14 2006-02-02 Toyota Motor Corp Fuel cell, manufacturing method therefor, and separator
US7749636B2 (en) 2004-09-21 2010-07-06 Reinz-Dichtungs-Gmbh Fuel cell arrangement and method of manufacturing a fuel cell arrangement
WO2006053236A1 (en) * 2004-11-12 2006-05-18 Trulite, Inc. Hydrogen generator cartridge
US20070154628A1 (en) * 2004-12-28 2007-07-05 Nissan Motor Co., Ltd. Solid polymer membrane fuel-cell manufacturing method
DE112006000172B4 (en) * 2005-01-10 2017-09-14 Dana Automotive Systems Group, Llc Fuel cell separator plate reinforcement via a connection assembly and method of manufacturing a bipolar fuel cell plate assembly
CN1858926A (en) * 2005-04-30 2006-11-08 比亚迪股份有限公司 Sealing device of proton exchanging film fuel cell unit
WO2007019172A2 (en) * 2005-08-03 2007-02-15 The University Of Alabama Silanes as a source of hydrogen
JP5130623B2 (en) * 2005-12-15 2013-01-30 トヨタ自動車株式会社 Fuel cell and gasket
ES2601053T3 (en) * 2006-01-17 2017-02-14 Henkel IP & Holding GmbH Joint fuel cell assembly and methods and systems to produce the same
JP4849931B2 (en) * 2006-03-29 2012-01-11 Nok株式会社 Seal structure
JP2007288701A (en) * 2006-04-20 2007-11-01 Hitachi Metals Ltd Irreversible circuit element
JP4978881B2 (en) 2006-06-26 2012-07-18 トヨタ自動車株式会社 Fuel cell
US7651542B2 (en) * 2006-07-27 2010-01-26 Thulite, Inc System for generating hydrogen from a chemical hydride
US7648786B2 (en) 2006-07-27 2010-01-19 Trulite, Inc System for generating electricity from a chemical hydride
US8357214B2 (en) * 2007-04-26 2013-01-22 Trulite, Inc. Apparatus, system, and method for generating a gas from solid reactant pouches
WO2009015331A1 (en) 2007-07-25 2009-01-29 Trulite, Inc. Apparatus, system, and method to manage the generation and use of hybrid electric power
KR101063461B1 (en) * 2008-10-15 2011-09-08 삼성전기주식회사 Fuel cell
DE102009014872A1 (en) 2009-03-30 2010-10-07 Lohmann Gmbh & Co. Kg Pressure-sensitive adhesive tape exhibiting a specific creep relaxation factor, useful as a sealing element in fuel cells
JP6168641B2 (en) * 2011-05-13 2017-07-26 日産自動車株式会社 Fuel cell
DE102012107753A1 (en) * 2012-08-22 2014-02-27 Windmöller & Hölscher Kg film product
EP2832812A1 (en) * 2013-07-29 2015-02-04 Nitto Shinko Corporation Sealant
GB201403551D0 (en) 2014-02-28 2014-04-16 Fujifilm Mfg Europe Bv Membrane stacks
JP2017157340A (en) * 2016-02-29 2017-09-07 住友電気工業株式会社 Redox flow cell

Family Cites Families (17)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
FR1593242A (en) * 1968-03-19 1970-05-25
JPS62280284A (en) * 1986-05-30 1987-12-05 Asahi Chem Ind Co Ltd Sealing member made of micro-cellular fluororesin foam
US4804451A (en) * 1986-10-01 1989-02-14 Millipore Corporation Depletion compartment for deionization apparatus and method
US5328816A (en) * 1988-09-13 1994-07-12 Canon Kabushiki Kaisha Process for producing optical recording medium
JPH079027B2 (en) * 1988-09-30 1995-02-01 住友金属工業株式会社 Forming method of low alloy steel for high temperature
US5284718A (en) * 1991-09-27 1994-02-08 Ballard Power Systems Inc. Fuel cell membrane electrode and seal assembly
JP3079742B2 (en) 1992-02-21 2000-08-21 富士電機株式会社 Solid polymer electrolyte fuel cell
JP3258390B2 (en) 1992-10-01 2002-02-18 三菱重工業株式会社 Fuel cell
JPH0765847A (en) * 1993-08-24 1995-03-10 Kansai Electric Power Co Inc:The Solid high polymer electrolyte type fuel cell
US5636098A (en) * 1994-01-06 1997-06-03 Applied Materials, Inc. Barrier seal for electrostatic chuck
JP3489181B2 (en) * 1994-03-10 2004-01-19 トヨタ自動車株式会社 Unit cell of fuel cell and method of manufacturing the same
JPH08148169A (en) * 1994-11-17 1996-06-07 Tokyo Gas Co Ltd Sealing method for solid polymeric fuel cell
JPH08185875A (en) * 1994-12-28 1996-07-16 Tokyo Gas Co Ltd Sealing method for solid high molecular fuel cell
JPH09199145A (en) * 1996-01-22 1997-07-31 Toyota Motor Corp Fuel cell and manufacture of fuel cell
DE19713250C2 (en) * 1997-03-29 2002-04-18 Ballard Power Systems Electrochemical energy converter with polymer electrolyte membrane
US6044842A (en) * 1997-05-19 2000-04-04 Pereira; Michael Gasketless connecting adapter
US5989741A (en) * 1997-06-10 1999-11-23 E.I. Du Pont De Nemours And Company Electrochemical cell system with side-by-side arrangement of cells

Also Published As

Publication number Publication date
JP3918265B2 (en) 2007-05-23
US6733916B2 (en) 2004-05-11
EP0918362A3 (en) 2004-12-22
JPH11154522A (en) 1999-06-08
US20010049047A1 (en) 2001-12-06
CA2253987C (en) 2003-04-01
EP0918362A2 (en) 1999-05-26

Similar Documents

Publication Publication Date Title
CA2253987A1 (en) Method of manufacturing fuel cells and fuel cells manufactured by the method
US7553577B2 (en) Sealing structure of fuel cell and process for molding rubber packing
US6660422B2 (en) Proton exchange membrane fuel cell external manifold seal
CA2279206A1 (en) Membrane-electrode unit with integrated sealing edge and method of making the same
EP1391956A1 (en) Fuel cell and method of manufacturing the fuel cell
US20060127738A1 (en) Design, method and process for unitized mea
WO2000002279A3 (en) Gas-proof assembly composed of a bipolar plate and a membrane-electrode unit of polymer electrolyte membrane fuel cells
US20020051902A1 (en) Method for mounting seals for fuel cell and fuel cell
JP2000156234A (en) Separator structure for fuel cell and its manufacture
CA2435098A1 (en) Seal structure of fuel cell unit and manufacturing method of the same
JP2005347255A (en) Unitized electrochemical battery semi-assembly, and manufacturing method of the same
CA2355700A1 (en) Gasket
CN102687330B (en) Fuel cell stack, manufacturing method of fuel cell stack and replacement method of module as constituent of fuel cell stack
US20030082430A1 (en) Fuel cell gasket assembly and method of making
WO2008114664A1 (en) Membrane-electrode bonding agent, proton conducting membrane with bonding layer, membrane-electrode assembly, solid polymer fuel cell, and method for producing membrane-electrode assembly
WO2005078839A3 (en) Method of forming bipolar plate modules
EP1482589A3 (en) Manufacturing process for membrane-electrode assemblies
JP2002056862A (en) Seal structure for fuel cell and method of forming rubber packing
EP1843419A1 (en) Adhesive sealing member and a fuel cell using the same
EP1737057A4 (en) Laminate-type cell, joining terminal, battery set, and process for producing battery set
JP4492770B2 (en) Fuel cell separator adhesive seal structure
EP2023424A3 (en) Alkaline dry battery and battery pack
JP3620294B2 (en) Sealing material for stacked fuel cell
JP3862210B2 (en) Fuel cell sealing structure and packing molding method
US8026019B2 (en) Fuel cell with proton exchange membrane bonded to acrylic plastic element

Legal Events

Date Code Title Description
EEER Examination request
MKLA Lapsed

Effective date: 20151112